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var cuttingPicParent=(true==true || true=="true") ?"1":"2"; var cuttingPicChild=(true==true || true=="true") ?"1":"2"; var definedDefaultImage=false; var defaultImage=(definedDefaultImage==true || definedDefaultImage=="true")?"/public/img/no-img.svg":""; var definedDefaultImageA=false; var defaultImageA=(definedDefaultImageA==true || definedDefaultImageA=="true")?"/public/img/no-img.svg":""; $comp({ config: { //用于描述此控件由多少個元素組成 item:{ //一級分類顯示項 level:[ {//定義此項是否顯示 show:false, //元素類型 type:"button", //元素樣式 key key:"button", //元素的值 v:"", //元素實例樣式依賴數據引用 depand:"open", //數據為false 值 depandStyleKey:"button1", //動作 action:{ //obj:當前對象,item 上面的配置參數,data 數據,config:element 配置 "click":function(scope,obj,item,data,config,itemConfig){ $.treeButtonClick(obj,config,item); } } }, { show:false, type:"thumb", key:"image", width:"30",//圖片位寬 height:"30",//圖片位高 errorImg:defaultImage, CuttingPic:cuttingPicParent,//圖片裁剪模式 1 裁剪 2普通（留白） //引用數據 img bindData:"icon" }, { show:true, type:"linkText", key:"linkText", //引用數據 name bindData:"name", config:{ //開關控制是否觸發顯示幾行操作 isShowLineNum:true, //顯示幾行 showlineNum:1 }, action:{ //obj:當前對象,item 上面的配置參數,data 數據,config:element 配置 "click":function(scope,obj,item,data,config,itemConfig){ $.treeButtonClick(obj,config,item,itemConfig); var openinNewWindow = data.targetType; if(openinNewWindow) { $.openNewWindow(data.linkUrl); }else{ $.openHref(data.linkUrl); } } } } /* , { show:true, type:"title", key:"num", //綁定數據源 bindData:"newsNum", float:"left" } */ ], //二級分類或子級分類顯示項 level1:[ { //定義此項是否顯示 show:false, //元素類型 type:"button", //元素樣式 key key:"button2", //元素的值 v:"", //元素實例樣式依賴數據引用 depand:"open", //數據為false 值 depandStyleKey:"button3", //動作 action:{ //obj:當前對象,item 上面的配置參數,data 數據,config:element 配置 "click":function(scope,obj,item,data,config){ $.treeButtonClick(obj,config,item); } } }, { show:true, type:"thumb", key:"imageA", width:"30",//圖片位寬 height:"30",//圖片位高 errorImg:defaultImageA, CuttingPic:cuttingPicChild,//圖片裁剪模式 1 裁剪 2普通（留白） //引用數據 img bindData:"icon" }, { show:true, type:"linkText", key:"linkText1", //引用數據 name bindData:"name", config:{ //開關控制是否觸發顯示幾行操作 isShowLineNum:true, //顯示幾行 showlineNum:1 }, action:{ "click":function(scope,obj,item,data,config){ var openinNewWindow = data.targetType; if(openinNewWindow) { $.openNewWindow(data.linkUrl) }else{ $.openHref(data.linkUrl); } } } } /* , { show:true, type:"title", key:"numA", //綁定數據源 bindData:"newsNum", float:"left" } */ ] }, //公共配置項 commonConfig:{ //深度 tree顯示幾層 //自定義子分類樣式 isDefindSubNode:false, //顯示子分類 isShowSubNode:false, //分類互斥展開 isExclusive:false, //無數據盒子 noData:"p_PromptNoneData", //盒子選中狀態 boxSelected:{ "zstyle":"p_box_selected", //綁定數據源 bindData:"selected" }, margin:{ show:false, left:"24", right:"24", bottom:"24", top:"24" } }, //元素配置參數 elements:{ //button 實例,圓點 dot:{ style:"e_icon-002", zstyle:"p_CategoryIconA" }, //一級線個性化 line:{ "style":"e_ListHline-001", "zstyle":"p_Listline" }, //leve1 線個性化 line1:{ "style":"e_ListHline-001", "zstyle":"p_ListlineA" }, //容器通用配置盒子容器 box:{ //頂層 "style":"e_box-000", "zstyle":"p_articles", //外層 out:{ "style":"e_box-000", "zstyle":"p_articlesA" }, //內層 inline:{ "style":"e_box-000", "zstyle":"p_articlesB" }, //一級配置 level:{ "style":"e_box-000", "zstyle":"p_articles", "out":{ "style":"e_box-000", "zstyle":"p_articlesA" }, "inline":{ "style":"e_box-000", "zstyle":"p_articlesB" } }, //二級配置 level1:{ "style":"e_box-000", "zstyle":"p_articles", "out":{ "style":"e_box-000", "zstyle":"p_articlesC" }, "inline":{ "style":"e_box-000", "zstyle":"p_articlesD" } } }, /***********以上配置項為必填***********/ //按鈕展開 class button:{ // "style":"e_icon-001", "zstyle":"p_CategoryIconZ" }, //按鈕收起class button1:{ "style":"e_icon-001", "zstyle":"p_CategoryIcon" }, //level1按鈕展開class + button2:{ "style":"e_icon-001", "zstyle":"p_CategoryIconZ" }, //level1 按鈕收起 class - button3:{ // "style":"e_icon-001", "zstyle":"p_CategoryIcon" }, // 縮略圖 data數據中必有img屬性 image:{ //效果class "style":"e_image-001", "zstyle":"p_image" }, // level1 imageA:{ //效果class "style":"e_image-001", "zstyle":"p_imageA" }, // ?? 鏈接文本數據中必有href name屬性或者有 total屬性 linkText:{ link:{ //效果class "style":"e_link-000", "zstyle":"p_link" }, text:{ //效果class "style":"e_MinorLink-001", "zstyle":"p_info" } }, //level1 鏈接文本1 linkText1:{ link:{ //效果class "style":"e_link-000", "zstyle":"p_link" }, text:{ //效果class "style":"e_MinorLink-001", "zstyle":"p_infoA" } }, //標題元素 num:{ "style":"e_AssistLabel-001", "zstyle":"p_num" }, //level 1 numA:{ "style":"e_AssistLabel-001", "zstyle":"p_numA" } }, //數據 //treeData:${cateTree} async:{ dataFilter: function(data){return data},//過濾器非必選 url:"/comp/news/categoryTree",//url路徑 autoParam:["id"],//動態參數 otherParam:{"selectId":selectId,"compId":"news_category-1535696339870","isAll":"false"}//靜態參數非必選 }, treeNode:["treeNode","treeNode1"]//模板（template） id } , params:{ definedDefaultImage:false, defaultImage:"/public/img/no-img.svg", definedDefaultImageA:false, defaultImageA:"/public/img/no-img.svg" }, //el等參數 id:"news_category-1535696339870",//實例id 服務器傳 lib:["js/news/news_category"] //組件js }); </script> </div></div> </div></div><div id="c_news_detail-15398787751722975" class="c_news_detail-01001"> <div class="e_box e_articles-001 p_NewsDetail "> <div class="e_box e_box-001 p_news">  <div class="e_box e_box-000 p_header">   <div class="e_box e_box-000 p_TitleBoxA"> <h1 class="e_title e_head-000 p_head "> <div class="font"> <i class="iconfont"></i> 貴金屬催化劑催化燃燒揮發性有機物(VOCs)：活性組分、載體性質等的影響 </div> </h1> </div> </div>   <div class="e_box e_box-000 p_AssistInfo"> <div class="e_box e_box-000 p_about">     </div> <div class="e_box e_box-000 p_InteractionInfo">  <div class="e_box e_box-000 p_ViewBox"> <div class="e_title e_AssistName-001 p_AssistNameE"> <div class="font"><i class="iconfont"></i><span class="i_browsingVolume">瀏覽量</span></div> </div> <div class="e_title e_AssistInfo-001 p_view" infoDetailId="638"> <div class="font"><i class="iconfont"></i></div> </div> </div>     </div> </div>  <div class="e_line e_ArticleHline-001 p_ArticleHline"></div>  <div class="e_box e_SummayBox-001 p_SummaryBox "> <div class="e_title e_name-001 p_nameC "> <div class="font"><i class="iconfont"></i> <span class="i_SummaryBox">【摘要】：</span></div> </div> <article class="e_article e_summary-001 p_summary"> 催化燃燒技術是目前處理揮發性有機物(VOCs)最有效的技術之一。在用于催化燃燒VOCs的催化劑中，貴金屬因其優異的催化活性而受到眾多關注。 </article> </div>   <div class="e_box e_box-000 p_content ">  <div class="e_box e_box-001 p_Atlas" data-innerdismoveable> <div> </div> </div>  <article class="e_HtmlEditor e_HtmlEditor-001 p_articles"> <div class="resetHtmlCssStyle"> <div class='reset_style js-reset_style js-adapMobile '><p> <span style="color: rgb(40, 40, 40); font-size: 14px; text-indent: 28px; background-color: rgb(193, 230, 198);"> 揮發性有機物(volatile organic compounds，VOCs)是指常溫下沸點為50～260 ℃的一系列有機化合物，是重要的大氣污染物。VOCs不僅參與光化學煙霧的形成，還可導致呼吸道和皮膚刺激，甚至誘使機體產生癌變，對環境和人體健康構成了很大威脅。因此，</span><a style="padding: 0px; margin: 0px; color: rgb(14, 106, 173); font-size: 14px; border: 0px; outline: none; text-indent: 28px; background-color: rgb(193, 230, 198);" target="_blank" title="VOCs處理新聞專題">VOCs處理</a><span style="color: rgb(40, 40, 40); font-size: 14px; text-indent: 28px; background-color: rgb(193, 230, 198);">技術日益受到重視。已開展應用的VOCs處理技術包括吸收法、吸附法、冷凝法、膜分離法、生化法、低溫等離子體法、光催化氧化法、直接燃燒法和催化燃燒法等。其中，催化燃燒法可以處理中、低濃度的VOCs，在相對較低的溫度下實現催化氧化，降低了能耗，減少了二次污染物的排放，目前已成為消除VOCs最重要的技術之一。</span></p> <div> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> <strong style="padding: 0px; margin: 0px;">一摘要</strong></p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 催化燃燒技術是目前處理揮發性有機物(VOCs)最有效的技術之一。在用于催化燃燒VOCs的催化劑中，貴金屬因其優異的催化活性而受到眾多關注。從活性組分和載體兩方面，對貴金屬催化劑催化燃燒VOCs的最新報道進行綜述。目前，催化劑活性組分的研究重點在于鉑、鈀、金等單組分貴金屬的改性和雙組分貴金屬的設計合成；對載體的研究主要涉及酸性、孔結構以及載體與金屬的強相互作用。未來還需進一步提高貴金屬催化劑的抗中毒性能。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> <strong style="padding: 0px; margin: 0px; text-indent: 28px;">二活性組分</strong></p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 1.Pt催化劑</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 總體上看，Pt催化劑對苯、甲苯具有較高的催化燃燒活性，在處理含氯VOCs時有更高的CO2選擇性，但難以催化氧化乙酸乙酯，且易受CO中毒的影響。對于Pt催化劑來說，隨著Pt顆粒尺寸的減小，Pt的分散度提升，Pt(0)的比例則下降，因而采用合適的方法，精確控制組分顆粒的尺寸，是改善催化性能的有效途徑。Chen等研究了一系列Pt顆粒尺寸在1.3～2.3 nm的Pt/ZSM-5對甲苯的催化燃燒性能，結果顯示，直徑為1.9 nm的Pt顆粒表現出了最佳的活性，因其較高分散度和高比例Pt(0)。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 過渡金屬改性的Pt催化劑是另一研究方向，過渡金屬的作用一般體現在兩方面：1)提高了Pt的分散度；2)與Pt產生協同作用，提升了活性和抗中毒性能。Zuo等研究發現：用稀土金屬Nd改性Pt/MCM-41后，貴金屬的分散度更高，催化燃燒苯的實驗顯示，Nd的添加使得Pt/MCM-41的T50由240 ℃降為200 ℃。Darif等研究表明：CuO和金屬Pt的相互作用能夠改善催化劑的抗硫穩定性， Pt-CuO/Al2O3催化劑在持續催化燃燒二甲基二硫醚30 h后，依然保持著相當的催化活性，催化劑在測試前后的起燃溫度T50無顯著差異。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 2.Pd催化劑</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 與Pt催化劑相比，Pd催化劑有更優異的水熱穩定性。在一定條件下，Pd催化劑擁有比Pt、Au催化劑更高的催化活性。Zhao等發現，Pd/CoAl-LDHs(層狀CoAl氫氧化物)中的PdO組分能夠活化載體上的氧物種，表現出對甲苯良好的催化燃燒性能，優于相同實驗條件下的Pt/CoAl-LDHs。Barakat等將Pd和Au分別負載到具有一定孔結構的CeTiO2載體上，對甲苯的催化燃燒實驗顯示，Pd/CeTiOx的起燃溫度T50為220 ℃，比Au/CeTiOx的起燃溫度T50低約70 ℃，并且在70 h的活性測試后依然保持著穩定的轉化率。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 負載方法顯著影響Pd催化劑性能的優劣。Liu等分別使用沉積沉淀法、前混合法和離子交換法制備Pd/OMS-2催化劑，性能評價結果顯示，用沉積沉淀法得到的Pd催化劑對甲苯和乙酸乙酯的催化燃燒活性均高于其余2種方法，原因在于沉積沉淀法能夠有效地避免活性物種的包埋，提升了表面Pd濃度和酸性位數量。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 3.Au催化劑</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> Au是一種對氧和氫呈現惰性的金屬，但Haruta等發現如將金屬態Au粒徑控制在5 nm以下，同時負載在金屬氧化物載體上，能夠顯著增強催化活性。相比于Pd和Pt，Au與吸附物間的作用力更為適中，在某些條件下能獲得遠優于Pt、Pd催化劑的效果。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> Au催化劑的研究重點在于載體的選擇以及Au與載體的協同效應。最近，Manzoli等觀察到Au與CoCe氧化物載體的協同作用，提升了活性氧的數量和催化反應能力。Yang等將納米Au浸漬到三維結構的MnOx/SiO2載體上，通過優化納米Au的負載比例，該催化劑對甲苯的起燃溫度T90可至255 ℃，提出了Au和MnOx納米顆粒間的相互作用是該催化劑高活性的原因之一。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 4.雙組分貴金屬催化劑</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 眾多研究表示，向單組分貴金屬催化劑中添加另一貴金屬組分，可促進電子的流動和表面氧的生成，影響顆粒粒徑和電子結構，展現了比單組分貴金屬催化劑更優異的催化活性。例如，Fu等在180 ℃下，用Pt-Pd/MCM-41雙組分貴金屬催化劑實現了對甲苯的完全氧化，該結果優于同等貴金屬含量的單組分催化劑(Pt/MCM-41和Pd/MCM-41)，分析顯示，該催化劑具有較高的表面Pt0含量和雙金屬協同作用導致的微小金屬顆粒。Guo等的研究結果顯示，Pt-Pd/TiOx比Pd/TiOx催化劑擁有更多的吸附氧物種，更有利于中間產物和吸附氧的輸送，從而加快氧化反應速率，提升催化活性。</p> <p style="padding: 0px; margin: 0px 0px 24px; border: 0px; font-size: 14px; color: rgb(40, 40, 40); text-indent: 2em; width: 620px; line-height: 24px; background-color: rgb(193, 230, 198);"> 稀土元素的加入能夠影響貴金屬原子表面的電荷轉移，進一步提升氧化還原能力，其中，CeO2在氧化還原過程中可快速實現Ce3+/Ce4+的轉變，常被用作催化助劑。Zuo等研究顯示，在高嶺土/NaY負載的Pd-Pt催化劑中加入Ce后，氧物種的數目增加，吸附氧溢流效應更加顯著，該催化劑對苯催化燃燒的T90為205 ℃，顯示出較好的催化反應活性。</p> </div> </div> </div> </article> </div> <div class="js_infoDetail_content item_hide"></div>   <div class="e_box e_box-000 p_assist">  </div>  <div class="e_line e_ArticleHline-001 p_ArticleHline"></div>  <div class="e_box e_box-000 p_PrevAndNext "> <div class="e_box e_box-000 p_previewBox"> <div class="e_title e_name-001 p_nameD "> <div class="font"><i class="iconfont"></i><span class="i_pageChangeUpTitle">上一篇：</span> </div> </div> <a href="/news/639.html" class="e_link e_link-000 p_LinkC"> <div class="e_title e_MinorLink-001 p_PreviewTitle" > <div class="font"><i class="iconfont"></i>保定市優環環?？萍加邢薰竟こ贪咐?/div> </div> </a> </div> <div class="e_box e_box-000 p_nextBox"> <a href="/news/637.html" class="e_link e_link-000 p_LinkD"> <div class="e_title e_MinorLink-001 p_PreviewTitle"> <div class="font"><i class="iconfont"></i>邢臺橡膠輪胎有機廢氣治理項目——15萬風量活性碳吸附+催化燃燒順利交工</div> </div> </a> <div class="e_title e_name-001 p_nameE "> <div class="font"><i class="iconfont"></i><span class="i_pageChangeDownTitle">下一篇：</span></div> </div> </div> </div>  </div> </div> <input type="hidden" id="infoTypeId" value="2"/> <input class="UrlParam" type="hidden" value="?id=638&type=0&cid=23&visualType=true" /> <input id="title_0" type="hidden" value="" /> <input id="desc_0" type="hidden" value="" /> <script> function scaleSplit(scale){ var sizearr=new Array(); 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